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Rutgers: The antidepressant drug sertraline repurposed?

Writer's picture: Ray SullivanRay Sullivan



George Carman is a Theobald Smith Society Past President (1997-1998) and Waksman Honorary Lecturer (1996).  His lab at the Rutgers Center for Lipid Research recently looked closely at the antidepressant drug sertraline and its possible use to remediate lipid-based disease.


Phosphatidic acid phosphatase (PAP) is an evolutionarily conserved eukaryotic enzyme that plays a key role in lipid homeostasis and is an important target for regulation to alleviate metabolic disorders associated with disturbances in phosphatidic acid and diacylglycerol levels.  Sertraline is a novel noncompetitive inhibitor of the Saccharomyces cerevisiae PAP enzyme Pah1 with an inhibition constant (Ki) of 13.5 μM, 7-fold lower than the commonly used PAP inhibitor propranolol.  Sertraline also inhibits the PAP activity of the human lipin 1 isoforms (α, β, and γ), with IC50 values approximately 2-fold lower than propranolol.  The inhibition of PAP activity by sertraline in yeast cells leads to a decrease in triacylglycerol content and an increase in phospholipid content, consistent with the role of PAP in regulating the balance between these lipid classes. 


PAP reaction and structures of sertraline and propranolol. A: PAP catalyzes the Mg2+-dependent dephosphorylation of PA to produce DAG. The structures of PA and DAG are shown with 16:0 and 18:1 acyl chains (B), the structure of sertraline. C: the structure of propranolol.
PAP reaction and structures of sertraline and propranolol. A: PAP catalyzes the Mg2+-dependent dephosphorylation of PA to produce DAG. The structures of PA and DAG are shown with 16:0 and 18:1 acyl chains (B), the structure of sertraline. C: the structure of propranolol.

They speculate that sertraline and/or structural analogs might be used to effect remediation of lipid-based disease based on PAP inhibition in humans to minimize latent Mycobacterium tuberculosis infection, alleviate intestinal inflammation-driven colon cancer development, suppress SARS-CoV-2 replication, and/or as an anti-mycotic.

 

Stukey GJ, Breuer MR, Burchat N, Jog R, Schultz K, Han GS, Sachs MS, Sampath H, Marmorstein R, Carman GM. The antidepressant drug sertraline is a novel inhibitor of yeast Pah1 and human lipin 1 phosphatidic acid phosphatases. J Lipid Res. 2025 Jan;66(1):100711. doi: 10.1016/j.jlr.2024.100711. Epub 2024 Nov 20. PMID: 39577771; PMCID: PMC11721541.  https://www.jlr.org/article/S0022-2275(24)00216-5/fulltext

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